Inverse modeling of past lead atmospheric deposition in South Greenland

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TitreInverse modeling of past lead atmospheric deposition in South Greenland
Type de publicationJournal Article
Year of Publication2015
AuteursMassa C, Monna F, Bichet V, Gauthier E, Losno R, Richard H
JournalATMOSPHERIC ENVIRONMENT
Volume105
Pagination121-129
Date PublishedMAR
Type of ArticleArticle
ISSN1352-2310
Mots-clésGreenland, inverse modeling, Lake, Lead stable isotopes, Peat, pollution
Résumé

The aim of this study is to model atmospheric lead fluxes in two different paleoenvironmental records located in southern Greenland. Fifty five sediment samples collected from the lake Igalilcu sedimentary sequence were analyzed for lead and aluminum concentrations, and lead isotopic compositions. The second archive consists in a previously published dataset, obtained from a minerogenic peat deposit, located at Tasiusaq, 16 km northwest from Lake Igaliku. A flux model fitted to both dataset produces similar results, allowing past anthropogenic atmospheric deposition to be reconstructed. This original method can be easily adapted for other studies where natural inputs dominate over discrete anthropogenic inputs. (C) 2015 Elsevier Ltd. All rights reserved.

DOI10.1016/j.atmosenv.2015.01.025